It looks like you have one of Delta's older 3530 models. Looking at the exploded diagram for this model shows part # H24 (the handle covers) with only a set screw holding it in place. If you've already removed that and the cover still won't lift off, it may be bound up on the stem from having been turned too far in one direction or the other (if it was leaking, I could imagine someone may have tried extra-hard to turn it off). I would try slowly but forcefully turning the faucet handle past its resistance point, with it in the on position first, then if that doesn't loosen it, try doing the same but the other direction with it in the off position. You may have to alternate this a few times to get it to free itself from the teeth on the stem.

If none of that works, there is a retaining nut on the underside of the sink counter (part # RP9519 in the diagram). It's not a very thick nut, so you'll have to put your hand right against the underside of the counter top to feel it. The threaded part of the stem assembly likely extends well past the nut, you'll need to make many turns to get it off. Taking the handle out from the counter will let you examine it in more detail and you can take tools to the less attractive parts to gain torque, hopefully avoiding any more scratches on the handle itself. Just be careful not to grip too tightly on the screw threads or you won't be able to reattach it to the counter!

Answer from CactusCake on Stack Exchange
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Plbg.com
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Removing shower handle on Delta 600 series
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It looks like you have one of Delta's older 3530 models. Looking at the exploded diagram for this model shows part # H24 (the handle covers) with only a set screw holding it in place. If you've already removed that and the cover still won't lift off, it may be bound up on the stem from having been turned too far in one direction or the other (if it was leaking, I could imagine someone may have tried extra-hard to turn it off). I would try slowly but forcefully turning the faucet handle past its resistance point, with it in the on position first, then if that doesn't loosen it, try doing the same but the other direction with it in the off position. You may have to alternate this a few times to get it to free itself from the teeth on the stem.

If none of that works, there is a retaining nut on the underside of the sink counter (part # RP9519 in the diagram). It's not a very thick nut, so you'll have to put your hand right against the underside of the counter top to feel it. The threaded part of the stem assembly likely extends well past the nut, you'll need to make many turns to get it off. Taking the handle out from the counter will let you examine it in more detail and you can take tools to the less attractive parts to gain torque, hopefully avoiding any more scratches on the handle itself. Just be careful not to grip too tightly on the screw threads or you won't be able to reattach it to the counter!

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It should just pull off. If it doesn't, you might try gently wiggling it side to side as you pull up. If you have a rubber or plastic mallet, you could try giving it a gentle tap to free it up. The trick is to be gentle enough to not break anything, but firm enough to knock it loose.

Discussions

replace Delta knob handle with lever handle in shower - DoItYourself.com Community Forums
Toilets, Sinks, Showers, Dishwashers, Tubs and Garbage Disposals - replace Delta knob handle with lever handle in shower - I have purchased a Delta conversion kit to replace my current shower knob handle with a lever handle. Because my tub spout was constantly dripping, an employee at Lowes ... More on doityourself.com
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October 29, 2010
Cannot remove Delta shower faucet
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Convert Delta faucet from Knob to Lever?? - DoItYourself.com Community Forums
Plumbing and Piping - Convert Delta faucet from Knob to Lever?? - In the house we just moved into the shower faucets are Delta brand with the clear knob handle. I'd like to convert the valve to a lever type control- anyone know if this is possible? Additionally, the existing valve trim is chrome ... More on doityourself.com
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January 26, 2010
Replacing Delta Faucet Acrylic Ball With A Lever Handle
You need this ball. https://www.lowes.com/pd/Danco-Stainless-Steel-Faucet-Or-Tub-Shower-Ball-Delta/1086479 You need this handle. https://www.lowes.com/pd/Danco-Chrome-Lever-Shower-Handle/1000296529 More on reddit.com
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